个人简介

　　杨汶醒，1988年生，2010年本科毕业于武汉理工大学，2012年硕士毕业于华南理工大学。2017年博士毕业于瑞典乌普萨拉大学，师从Gerrit Boschloo教授和瑞典科学院、工程院院士Anders Hagfeldt教授。2017-2018年在英国帝国理工大学开展博士后研究，师从英国皇家学会院士James R. Durrant 教授。2018-2021年，赴美国埃默里大学开展博后研究工作，师从知名超快光谱专家Tianquan Lian教授。2021年9月入职西湖大学理学院，人工光合作用与太阳能燃料中心，组建光谱与催化机制实验室，任特聘研究员（独立PI/博士生导师）。

学术成果

杨汶醒博士长期致力于光催化、电催化、光电催化过程中的时间分辨光谱和原位光谱研究。通过结合原位电化学光谱（红外、拉曼）、超快光谱等谱学手段和结构表征技术，探索催化剂表面结构、活性位点与化学键断裂、结合之间的构效关系, 旨在促进太阳能转化技术的发展，推动光电催化关键科学问题的新认知。近年来在国际知名学术期刊发表论文30余篇，其中第一和通讯作者论文15篇，包括Nat. Commun., J. Am. Chem. Soc., Nano. Lett., Chem. Sci., ACS Energy Lett.等。2017年博士论文获瑞典乌普萨拉大学Bjurzons premium奖。2018年获德国洪堡学者资助邀请。2018-2021年独立主持瑞典基金理事会基金用于纳米晶人工光合作用的电子转移研究。现主持国家自然科学基金面上项目，作为课题骨干参与科技部重点研发项目。担任多个学术期刊审稿人，担任Wiley-VCH 旗下杂志Chemistry-Method的Early career advisory board members.

代表论文（*代表通信作者）

1. Li, Z; Wang, L.; Sun, L.; Yang, W.*, Dynamic Cation Enrichment During Pulsed CO2 Electrolysis and the Cation-Promoted Multicarbon Formation. J. Am. Chem. Soc. 2024, doi.org/10.1021/jacs.4c06404

2. Chen, H.†; Zhao, W.†;  Wang, L.; Chen, Z.; Ye, W.; Zang, J.; Wang, T.*; Sun, L.; Yang, W.*, Origin of Metal−Support Interactions for Selective Electrochemical CO2 Reduction into C1 and C2+ Products. ACS Catal. 2024, doi.org/10.1021/acscatal.4c02335

3. Sun, R; Zang, J.; Lai, R.; Yang, W.*, Ji, B.*, Near-Infrared-to-Visible Photon Upconversion with Efficiency Exceeding 21% Sensitized by InAs Quantum Dots. J. Am. Chem. Soc. 2024, 146, 26, 17618–17623.

4. Liu, Q; Jiang, Q.; Li, L.; Yang, W.*, Spontaneous Reconstruction of Copper Active Sites during the Alkaline CORR: Degradation and Recovery of the Performance.  J. Am. Chem. Soc. 2024, 146, 6, 4242–4251.

5. Li, Z.; Wang, L.; Wang, T.; Sun, L.; Yang, W.*, Steering the Dynamics of Reaction Intermediates and Catalyst Surface during Electrochemical Pulsed CO₂ Reduction for Enhanced C₂₊ Selectivity. J. Am. Chem. Soc. 2023, 145 (37), 20655-20664. 

(Highlighted in Nature Chemistry, https://www.nature.com/articles/s41557-023-01371-2)

6. Liu, Y.; Yang, W.*; Chen, Q.; Cullen, D.; Xie, Z.; Lian, T.; * PT Particle Size Affects Both the Charge Separation and Water Reduction Efficiencies of CdS-Pt Nanorod Photocatalysts for Light Driven H₂ Generation. J. Am. Chem. Soc. 2022, 144(6), 2705–2715.

7. Yang, W.; Godin, R.; Kasap, H.; Moss, B.; Dong, Y.; Hillman, S. A. J.; Steier, L.; Reisner, E.; Durrant, J. R.* Electron Accumulation Induces Efficiency Bottleneck for Hydrogen Production in Carbon Nitride Photocatalysts. J. Am. Chem. Soc. 2019, 141 (28), 11219–11229.

8. Yang, W.*; Liu, Y.; Cullen, D. A; McBride, J. R.; Lian, T.* Harvesting Sub-bandgap IR Photons by Photo-thermionic Hot Electron Transfer in a Plasmonic p-n junction, Nano Lett 2021, 21, 9, 4036–4043

9. Yang, W.; Liu, Y.; Edvinsson, T; Castner, A; Wang, S; He. S; Ott, S; Hammarström, L*, Lian, T.*. Photoinduced Fano Resonances between Quantum Confined Nanocrystals and Adsorbed Molecular Catalysts, Nano Lett. 2021, 21, 13, 5813–5818

10. Yang, W.*†; Liu, Y.†; McBride, J. R.; Lian, T.* Ultrafast and Long-lived Transient Heating of Surface Adsorbates on Plasmonic Semiconductor Nanocrystals, Nano Lett 2021, 21, 453-461.

11. Yang, W.*; Yang, Y.; Kaledin, A. L.; He, S.; McBride, J. R.; Lian, T.* Surface Passivation Extends Single and Biexciton Lifetimes of InP Quantum Dots. Chemical Science, 2020,11, 5779-5789.

12. Yang, W.*; Vlachopoulos, N.; Boschloo, G. Impact of Local Electric Fields on Charge-Transfer Processes at the TiO₂ /Dye/Electrolyte Interface. ACS Energy Lett. 2017, 2 (1), 161–167.

13. Yang, W.*; Vansuch, G., Liu, Y., Jin, T., Liu, Q.; Ge, A., Monica, S., Sanchez, M. L. K; Adams, M. W. W.; Dyer, R. B.*, Lian, T.* “Liquid” to “crystalline” phase transition of surface ligands modulate the quantum efficiency of H₂ production in mediator based CdS nanorod/Hydrogenases assemblies. ACS Applied Material and Interfaces, 2020, 12, 31, 35614–35625.

14. Yang, W.; Hao, Y.*; Kloo, L.; Boschloo, G.* Carrier Dynamics of Dye-Sensitized TiO₂ in Contact with Different Cobalt Complexes in the Presence of Tri(p-Anisyl)Amine Intermediates. J. Phys. Chem. C 2018, 122 (26), 14345–14354.

15. Yang, W.*; Hao, Y.; Vlachopoulos, N.; Eriksson, A. I. K.; Boschloo, G.* Studies on the Interfacial Electric Field and Stark Effect at the TiO₂/Dye/Electrolyte Interface. J. Phys. Chem. C 2016, 120 (39), 22215–22224.

16. Yang, W.; Pazoki, M.; Eriksson, A. I. K.; Hao, Y.; Boschloo, G. A Key Discovery at the TiO₂/Dye/Electrolyte Interface: Slow Local Charge Compensation and a Reversible Electric Field. Phys. Chem. Chem. Phys. 2015, 17 (26), 16744–16751.

Google Scholar:

https://scholar.google.com/citations?user=ySLroqgAAAAJ

Research Gate:

https://www.researchgate.net/profile/Wenxing-Yang

联系方式

电子邮箱：yangwenxing@westlake.edu.cn

杨汶醒博士课题组目前的主要重点研究包括但不限于：

1. 电催化水氧化、CO2还原、N2还原的原位谱学和催化机制；

2. 大电流膜电极器件的设计和原位表征；

3. 高时空分辨原位谱学技术的研发；

4. 高效光电催化剂的超快光谱和激发态动力学；